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Processing app for mass-spectrometric CO₂ clumped isotope (∆₄₇, ∆₄₈ and ∆₄₉) data.

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Welcome to D4Xgui v1.0.2!

D4Xgui is developed to enable easy access to state-of-the-art CO₂ clumped isotope (∆₄₇, ∆₄₈ and ∆₄₉) data processing. A recently developed optimizer algorithm allows pre-processing of mass spectrometric raw intensities utilizing a m/z47.5 half-mass Faraday cup correction to account for the effect of a negative pressure baseline, which is essential for accurate and highest precision clumped isotope analysis of CO₂ (Bernecker et al., 2023). It is backed with the recently published processing tool D47crunch (v.2.4.3) (following the methodology outlined in Daeron, 2021), which allows standardization under consideration of full error propagation and has been used for the InterCarb community effort (Bernasconi et al., 2021). This web-app allows users to discover replicate- or sample-based processing results in interactive spreadsheets and plots.


Example data is accessible from the Data-IO page, or can be downloaded from GitHub. Please check INSTALLATION.md to find help setting up D4Xgui.


In order to process post-background corrected data (Data-IO page, Upload δ⁴⁵-δ⁴⁹ replicates tab), the following columns need to be provided (.xlsx, .csv):

UID Sample Session Timetag d45 d46 d47 d48 d49

$~$

Baseline correction can be performed using a m/z47.5 half-mass cup. For this purpose either a set of equilibrated gases (via heated-gas-line), or carbonate standards (via target values) is used to determine m/z47, m/z48 and m/z49-specific scaling factors. Please upload a cycle-based spreadsheet (.xlsx, .csv) including the following columns (Data-IO page, Upload m/z44-m/z49 intensities tab):

UID Sample Session Timetag Replicate
raw_r44 raw_r45 raw_r46 raw_r47 raw_r48 raw_r49 raw_r47.5
raw_s44 raw_s45 raw_s46 raw_s47 raw_s48 raw_s49 raw_s47.5



Please find the code documentation here.

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Processing app for mass-spectrometric CO₂ clumped isotope (∆₄₇, ∆₄₈ and ∆₄₉) data.

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